Abstract The performance of aqueous zinc‐ion batteries (AZIBs) at high temperatures (HT) is severely compromised by active water corrosion, parasitic reactions, and dendrite growth. Herein, zinc trifluoroacetate is introduced at a low concentration (0.2 m ), dissolved in triethyl phosphate (TEP)and H 2 O. The active water is suppressed due to the reconstructed original hydrogen bond network, which helps inhibit parasitic reactions and severe corrosion. Meanwhile, a solid electrolyte interphase (SEI) formed on the zinc anode due to the decomposition of the introduced zinc salt. The high‐tolerance SEI physically separates the electrolyte and anode, reducing the corrosion caused by active water. Moreover, TEP, as a prevalent fire‐retardant cosolvent, can preferentially anchor on the zinc sheet, serving as a shielding buffer layer. TEP is not only reconstructing the structure of the electric double layer (EDL), decreasing the content of active water, but also accelerating the prompt formation of SEI further. As proof of this synergistic effect, the assembled symmetric Zn.

Changlei Zhuang

Siwen Zhang

Zhi Gen Yu

Jinzhang Yang

Ying Sun

Hanyu Wen

Haokun Wen

Hui Li

Bosi Yin

Tianyi Ma

Advanced Functional Materials

作为顶级材料科学期刊，ADVANCED FUNCTIONAL MATERIALS 每周报道材料科学各个方面的突破性研究，包括纳米技术、化学、物理和生物学。ADVANCED FUNCTIONAL MATERIALS 以其快速和公平的同行评审、质量而闻名内容丰富，影响力大，成为国际材料科学界的首选。主题：材料科学、纳米技术、液晶、半导体、超导体、光学、激光、传感器、多孔材料、发光材料、陶瓷、生物材料、磁性材料、薄膜、胶体、先进、材料、能源材料。

Advanced Functional Materials is a leading journal in materials science that publishes groundbreaking research across various aspects of the field on a weekly basis, including nanotechnology, chemistry, physics, and biology. Renowned for its rapid and fair peer review process and high-quality content, it has become the preferred choice in the international materials science community. Key topics covered include materials science, nanotechnology, liquid crystals, semiconductors, superconductors, optics, lasers, sensors, porous materials, luminescent materials, ceramics, biomaterials, magnetic materials, thin films, colloids, advanced materials, and energy materials.

《Advanced Functional Materials》是顶尖的材料科学期刊，每周报道材料科学领域的最新突破，包括纳米技术、化学、物理和生物学等方面。该期刊以其快速而公正的同行评审和高质量的内容而闻名，成为国际材料科学界的首选。主要主题包括：材料科学、纳米技术、液晶、半导体、超导体、光学、激光、传感器、多孔材料、发光材料、陶瓷、生物材料、磁性材料、薄膜、胶体、先进材料和能源材料。

Category	Quartile
材料科学	1
材料科学, 化学综合	1
材料科学, 物理化学	1
材料科学, 材料科学综合	1
材料科学, 纳米科技	1
材料科学, 物理应用	1
材料科学, 物理凝聚态物理	1

Synergistic Effect Enables Aqueous Zinc‐Ion Batteries to Operate at High Temperatures

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Journal Info

Category	Quartile
PHYSICS, CONDENSED MATTER	1